Photonics and Lasers

Chapter 9 - Nonlinear Optics

Chapter 9

 

Nonlinear Optics

In the preceding chapters we have assumed that light interacts with matter in a linear fashion. A linear interaction is illustrated in Fig. 9-1a, which shows two light waves of different frequency intersecting in a material medium. The presence of wave 2 has no affect on wave 1, and vice versa. The waves are uncoupled, and propagate independently. In contrast, a nonlinear interaction is characterized by a coupling of two or more intersecting waves, as illustrated in Fig. 9-1b. In this case, each wave can modify the properties of the other, changing, for example, the other wave's amplitude or phase. One of the waves can also modify its own amplitude or phase, a phenomenon termed self-action. Still another possibility in a nonlinear interaction is the generation of new waves with a frequency different from those of the incident beams. This frequency conversion process does not occur in a linear medium.

In a perfect vacuum, there is no coupling between two light waves because Maxwell's equations (which govern the propagation of an electromagnetic wave) are linear in the electric and magnetic field variables. The superposition principle then applies, which states that the sum of two solutions is itself another solution to the equations. Coupling between two light waves is only allowed when light propagates in a material medium, and it is an indirect type of process. One wave changes the properties of the medium in some way, and then the second wave is affected by the changed properties of the medium. The degree of coupling between two light waves, therefore, depends on how strongly the light wave interacts with the medium.

The interaction between light and matter is normally quite weak. The order of magnitude of this interaction can be estimated by comparing the strength of the light wave's electric field E to the electric field Eain the atoms of the material. Light from the sun, for example, has a typical field E 600 V/m, whereas typical atomic fields are Ea ~ 1011 V/m (see Problem 9.1). Since E Ea, the light wave deviates the electrons in the material only slightly from their normal positions, which means that the light-matter interaction is weak. It is actually a good thing that nonlinear optical effects are usually negligible, because linear behavior is necessary for the image-forming property of lenses. To form a proper image, light from each point of an object must propagate to the image plane in a manner that does not depend on the presence or absence of light from other points on the object, which is simultaneously passing through the lens. Nonlinear interactions would cause a distorted image.

Nonlinear effects are expected to become important only for very high optical intensity I, where the field E (given by Eq. 2-9) is large. It is therefore not surprising that the development of lasers, which are capable of very high intensities, has spurred on progress in understanding and applying nonlinear optical phenomena. Indeed, the first important experimental demonstration of nonlinear optics, that of second-harmonic generation by Franken and coworkers in 1961, occurred just after the demonstration of the first laser in

09_Photonics_and_Lasers-1.jpg


09_Photonics_and_Lasers-2.jpg

Figure 9-1 (a) In a linear medium, two waves pass through the same region of space without interacting, (b) In a nonlinear medium, two waves that overlap spatially may each modify the properties of the other, and create additional waves with different frequencies.

1960. Since that time, laser physics and nonlinear optics have matured into two rich and multifaceted subdisciplines, each evolving in synergy with the other. Today, they are inextricably linked, lasers being needed to study nonlinear effects, and nonlinear effects being needed for the operation of many lasers.

In this introductory survey, space permits us to sample just a few of the many diverse aspects of nonlinear optics. After first reviewing the mechanisms that give rise to nonlinear effects, we next consider those phenomena in which new frequencies are generated, and then those in which the frequency remains unchanged, but some other property (such as phase) is modified. Finally, we consider the electrooptic effects, in which the optical properties of a material are modified by a static electric field. More complete treatments of these and other nonlinear optical phenomena will be found in the Bibliography.

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